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The project aims to develop new approaches for investigation of reaction mechanisms in photocatalytic reactions. As a PhD Candidate you will learn and then improve our strategies to trap reaction intermediates in photocatalytic reactions by mass spectrometry. The initial studies will concern C-H activation and oxidation reactions mediated by metal complexes as photocatalysts. Understanding of key reaction steps and identification of reaction intermediates will be a guide towards developing of improved photocatalysts. The project will run within the frame NWO START-UP Grant of Prof. Roithova. For relevant literature see: Acc. Chem. Res. 2016, 49, 223; J. Am. Chem. Soc. 2017, 139, 2757; Phys. Chem. Chem. Phys. 2018, 20, 6868.
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Faculty of Science
The research project will be carried out by Prof. Roithova’s group at the Institute for Molecules and Materials of Radboud University (Nijmegen, Netherlands). Prof. Roithova’s group is housed in the Huygens building with access to chemical laboratories, all standard analytical equipment, and a computer cluster for theoretical calculations. In addition, the group is equipped with a cryotrapping ion spectroscopy experiment, IR and UV-vis OPOs and several mass spectrometers dedicated to mechanistic research.
Further information on Roithová Group
Further information on Spectroscopy & Catalysis
Further information on M-O Bonding Beyond the Oxo Wall: Spectroscopy and Reactivity of Cobalt(III)-Oxyl and Cobalt(III)-Oxo Complexes (open access)
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